面向行业关键技术需求，紧密围绕 “煤代油”路线的“甲醇制烯烃”关键工业步骤，从事分子筛多孔材料催化甲醇等C1化学分子转化的基础研究

081705-工业催化

分子筛催化剂，催化反应机理

   

博士研究生

博士

   

2019-01~现在, 大连化学物理研究所, 副研究员/工学博士

   

（1） 辽宁省自然科学学术成果奖, 一等奖, 省级, 2018

（ 1 ） 一种金属改性SAPO-34分子筛的制备方法, 发明专利, 2021, 第 1 作者, 专利号: CN110902693B

   

[1] Wu,xinqiang. Dynamic catalytic mechanism of methanol to hydrocarbons reaction over zeolite. Accounts of chemical research[J]. 2023, [2] Xinqiang Wu, Wei Chen, Shutao Xu, Shanfan Lin, Tantan Sun, Anmin Zheng, Yingxu Wei, Zhongmin Liu. Dynamic Activation of C1 Molecules Evoked by Zeolite Catalysis. ACS CENTRAL SCIENCE[J]. 2021, 7(4): 681-687, https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8155459/.
[3] Lin, Shanfan, Zhi, Yuchun, Chen, Wei, Li, Huan, Zhang, Wenna, Lou, Caiyi, Wu, Xinqiang, Zeng, Shu, Xu, Shutao, Xiao, Jianping, Zheng, Anmin, Wei, Yingxu, Liu, Zhongmin. Molecular Routes of Dynamic Autocatalysis for Methanol-to-Hydrocarbons Reaction. JOURNAL OF THE AMERICAN CHEMICAL SOCIETY[J]. 2021, 143(31): 12038-12052, http://dx.doi.org/10.1021/jacs.1c03475.
[4] Yu, Bowen, Zhang, Wenna, Wei, Yingxu, Wu, Xinqiang, Sun, Tantan, Fan, Benhan, Xu, Shutao, Liu, Zhongmin. Capture and identification of coke precursors to elucidate the deactivation route of the methanol-to-olefin process over H-SAPO-34. CHEMICAL COMMUNICATIONS[J]. 2020, 56(58): 8063-8066, https://www.webofscience.com/wos/woscc/full-record/WOS:000550563800010.
[5] Zhang, Wenna, Zhi, Yuchun, Huang, Jindou, Wu, Xinqiang, Zeng, Shu, Xu, Shutao, Zheng, Anmin, Wei, Yingxu, Liu, Zhongmin. Methanol to Olefins Reaction Route Based on Methylcyclopentadienes as Critical Intermediates. ACS CATALYSIS[J]. 2019, 9(8): 7373-7379, https://www.webofscience.com/wos/woscc/full-record/WOS:000480503700080.
[6] Gao, Shushu, Xu, Shutao, Wei, Yingxu, Qiao, Qinglong, Xu, Zhaochao, Wu, Xinqiang, Zhang, Mozhi, He, Yanli, Xu, Shuliang, Liu, Zhongmin. Insight into the deactivation mode of methanol-to-olefins conversion over SAPO-34: Coke, diffusion, and acidic site accessibility. JOURNAL OF CATALYSIS[J]. 2018, 367: 306-314, http://dx.doi.org/10.1016/j.jcat.2018.09.010.
[7] Wu, Xinqiang, Xu, Shutao, Wei, Yingxu, Zhang, Wenna, Huang, Jindou, Xu, Shuliang, He, Yanli, Lin, Shanfan, Sun, Tantan, Liu, Zhongmin. Evolution of C-C Bond Formation in the Methanol-to-Olefins Process: From Direct Coupling to Autocatalysis. ACS CATALYSIS[J]. 2018, 8(8): 7356-7361, https://www.webofscience.com/wos/woscc/full-record/WOS:000441112400056.
[8] Zhang, Wenna, Chen, Jingrun, Xu, Shutao, Chu, Yueying, Wei, Yingxu, Zhi, Yuchun, Huang, Jindou, Zheng, Anmin, Wu, Xinqiang, Meng, Xiangju, Xiao, Fengshou, Deng, Feng, Liu, Zhongmin. Methanol to Olefins Reaction over Cavity-type Zeolite: Cavity Controls the Critical Intermediates and Product Selectivity. ACS CATALYSIS[J]. 2018, 8(12): 10950-10963, http://www.corc.org.cn/handle/1471x/2372921.
[9] Xu, Shutao, Zhi, Yuchun, Han, Jingfeng, Zhang, Wenna, Wu, Xinqiang, Sun, Tantan, Wei, Yingxu, Liu, Zhongmin, Song, C. Advances in Catalysis for Methanol-to-Olefins Conversion. ADVANCES IN CATALYSIS, VOL 61null. 2017, 61: 37-122, https://www.webofscience.com/wos/woscc/full-record/WOS:000432515600003.
[10] Wu, Xinqiang, Xu, Shutao, Zhang, Wenna, Huang, Jindou, Li, Jinzhe, Yu, Bowen, Wei, Yingxu, Liu, Zhongmin. Direct Mechanism of the First Carbon-Carbon Bond Formation in the Methanol-to-Hydrocarbons Process. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION[J]. 2017, 56(31): 9039-9043, https://www.webofscience.com/wos/woscc/full-record/WOS:000424260200016.
[11] Zhang, Mozhi, Xu, Shutao, Li, Jinzhe, Wei, Yingxu, Gong, Yanjun, Chu, Yueying, Zheng, Anmin, Wang, Jinbang, Zhang, Wenna, Wu, Xinqiang, Deng, Feng, Liu, Zhongmin. Methanol to hydrocarbons reaction over H beta zeolites studied by high resolution solid-state NMR spectroscopy: Carbenium ions formation and reaction mechanism. JOURNAL OF CATALYSIS[J]. 2016, 335: 47-57, http://ir.wipm.ac.cn/handle/112942/9198.
[12] 王金棒, 李金哲, 徐舒涛, 郅玉春, 魏迎旭, 何艳丽, 陈景润, 张默之, 王全义, 张雯娜, 武新强, 郭新闻, 刘中民. HZSM-22和SAPO-11催化甲醇转化制烯烃（MTH）反应：酸强度对反应和失活机理的影响. 催化学报[J]. 2015, 36(8): 1392-1402, http://lib.cqvip.com/Qikan/Article/Detail?id=665710049.
[13] Wang Jinbang, Li Jinzhe, Xu Shutao, Zhi Yuchun, Wei Yingxu, He Yanli, Chen Jingrun, Zhang Mozhi, Wang Quanyi, Zhang Wenna, Wu Xinqiang, Guo Xinwen, Liu Zhongmin. HZSM-22和SAPO-11催化甲醇转化制烯烃（MTH）反应：酸强度对反应和失活机理的影响. 催化学报[J]. 2015, 36(8): 1392-1402, http://lib.cqvip.com/Qikan/Article/Detail?id=665710049.
[14] Wang, Jinbang, Li, Jinzhe, Xu, Shutao, Zhi, Yuchun, Wei, Yingxu, He, Yanli, Chen, Jingrun, Zhang, Mozhi, Wang, Quanyi, Zhang, Wenna, Wu, Xinqiang, Guo, Xinwen, Liu, Zhongmin. Methanol to hydrocarbons reaction over HZSM-22 and SAPO-11: Effect of catalyst acid strength on reaction and deactivation mechanism. CHINESE JOURNAL OF CATALYSIS[J]. 2015, 36(8): 1392-1402, http://dx.doi.org/10.1016/S1872-2067(15)60953-6.
[15] 王金棒, 李金哲, 徐舒涛, 郅玉春, 魏迎旭, 何艳丽, 陈景润, 张默之, 王全义, 张雯娜, 武新强, Xinwen Guo, 刘中民. Methanol to hydrocarbons reaction over HZSM-22 and SAPO-11: Effect of catalyst acid strengthon reaction and deactivation mechanism. CHINESE JOURNAL OF CATALYSIS催化学报[J]. 2015, 36: 1392-, http://cas-ir.dicp.ac.cn/handle/321008/148156.

   

（ 1 ） 原位谱学技术研究分子筛催化甲醇转化反应诱导期的自催化作用机制, 负责人, 国家任务, 2020-01--2022-12
（ 2 ） “优秀青年博士人才”, 负责人, 研究所自选, 2019-01--2023-12