面向行业关键技术需求，紧密围绕 “煤代油”路线的“甲醇制烯烃”关键工业步骤，从事分子筛多孔材料催化甲醇等C1化学分子转化的基础研究

081705-工业催化

分子筛催化剂，催化反应机理

   

博士研究生

博士

   

2019-01~现在, 大连化学物理研究所, 副研究员/工学博士

   

（1） 辽宁省自然科学学术成果奖, 一等奖, 省级, 2018

（ 1 ） 一种金属改性SAPO-34分子筛的制备方法, 发明专利, 2021, 第 1 作者, 专利号: CN110902693B

   

[1] Wu, Xinqiang, Wei, Yingxu, Liu, Zhongmin. Dynamic Catalytic Mechanism of the Methanol-to-Hydrocarbons Reaction over Zeolites. ACCOUNTS OF CHEMICAL RESEARCH. 2023, 第 1 作者56(14): 2001-2014, http://dx.doi.org/10.1021/acs.accounts.3c00187.
[2] Wang, Nan, Wang, Li, Zhi, Yuchun, Han, Jingfeng, Zhang, Chengwei, Wu, Xinqiang, Zhang, Jinling, Wang, Linying, Fan, Benhan, Xu, Shutao, Zheng, Yijun, Lin, Shanfan, Wu, Renan, Wei, Yingxu, Liu, Zhongmin. Coking and decoking chemistry for resource utilization of polycyclic aromatic hydrocarbons (PAHs) and low-carbon process. JOURNAL OF ENERGY CHEMISTRY[J]. 2023, 第 6 作者76: 105-116, http://dx.doi.org/10.1016/j.jechem.2022.09.014.
[3] Xinqiang Wu, Wei Chen, Shutao Xu, Shanfan Lin, Tantan Sun, Anmin Zheng, Yingxu Wei, Zhongmin Liu. Dynamic Activation of C1 Molecules Evoked by Zeolite Catalysis. ACS CENTRAL SCIENCE[J]. 2021, 第 1 作者7(4): 681-687, https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8155459/.
[4] Lin, Shanfan, Zhi, Yuchun, Chen, Wei, Li, Huan, Zhang, Wenna, Lou, Caiyi, Wu, Xinqiang, Zeng, Shu, Xu, Shutao, Xiao, Jianping, Zheng, Anmin, Wei, Yingxu, Liu, Zhongmin. Molecular Routes of Dynamic Autocatalysis for Methanol-to-Hydrocarbons Reaction. JOURNAL OF THE AMERICAN CHEMICAL SOCIETY[J]. 2021, 第 7 作者143(31): 12038-12052, http://dx.doi.org/10.1021/jacs.1c03475.
[5] Sun, Tantan, Chen, Wei, Xu, Shutao, Zheng, Anmin, Wu, Xinqiang, Zeng, Shu, Wang, Nan, Meng, Xiangju, Wei, Yingxu, Liu, Zhongmin. The first carbon-carbon bond formation mechanism in methanol-to-hydrocarbons process over chabazite zeolite. CHEM[J]. 2021, 第 5 作者7(9): 2415-2428, http://dx.doi.org/10.1016/j.chempr.2021.05.023.
[6] Yu, Bowen, Zhang, Wenna, Wei, Yingxu, Wu, Xinqiang, Sun, Tantan, Fan, Benhan, Xu, Shutao, Liu, Zhongmin. Capture and identification of coke precursors to elucidate the deactivation route of the methanol-to-olefin process over H-SAPO-34. CHEMICAL COMMUNICATIONS[J]. 2020, 第 4 作者56(58): 8063-8066, https://www.webofscience.com/wos/woscc/full-record/WOS:000550563800010.
[7] Zhang, Wenna, Zhi, Yuchun, Huang, Jindou, Wu, Xinqiang, Zeng, Shu, Xu, Shutao, Zheng, Anmin, Wei, Yingxu, Liu, Zhongmin. Methanol to Olefins Reaction Route Based on Methylcyclopentadienes as Critical Intermediates. ACS CATALYSIS[J]. 2019, 第 4 作者9(8): 7373-7379, https://www.webofscience.com/wos/woscc/full-record/WOS:000480503700080.
[8] Gao, Shushu, Xu, Shutao, Wei, Yingxu, Qiao, Qinglong, Xu, Zhaochao, Wu, Xinqiang, Zhang, Mozhi, He, Yanli, Xu, Shuliang, Liu, Zhongmin. Insight into the deactivation mode of methanol-to-olefins conversion over SAPO-34: Coke, diffusion, and acidic site accessibility. JOURNAL OF CATALYSIS[J]. 2018, 第 6 作者367: 306-314, http://dx.doi.org/10.1016/j.jcat.2018.09.010.
[9] Wu, Xinqiang, Xu, Shutao, Wei, Yingxu, Zhang, Wenna, Huang, Jindou, Xu, Shuliang, He, Yanli, Lin, Shanfan, Sun, Tantan, Liu, Zhongmin. Evolution of C-C Bond Formation in the Methanol-to-Olefins Process: From Direct Coupling to Autocatalysis. ACS CATALYSIS[J]. 2018, 第 1 作者8(8): 7356-7361, https://www.webofscience.com/wos/woscc/full-record/WOS:000441112400056.
[10] Zhang, Wenna, Chen, Jingrun, Xu, Shutao, Chu, Yueying, Wei, Yingxu, Zhi, Yuchun, Huang, Jindou, Zheng, Anmin, Wu, Xinqiang, Meng, Xiangju, Xiao, Fengshou, Deng, Feng, Liu, Zhongmin. Methanol to Olefins Reaction over Cavity-type Zeolite: Cavity Controls the Critical Intermediates and Product Selectivity. ACS CATALYSIS[J]. 2018, 第 9 作者8(12): 10950-10963, http://www.corc.org.cn/handle/1471x/2372921.
[11] Xu, Shutao, Zhi, Yuchun, Han, Jingfeng, Zhang, Wenna, Wu, Xinqiang, Sun, Tantan, Wei, Yingxu, Liu, Zhongmin, Song, C. Advances in Catalysis for Methanol-to-Olefins Conversion. ADVANCES IN CATALYSIS, VOL 61. 2017, 第 5 作者61: 37-122, https://www.webofscience.com/wos/woscc/full-record/WOS:000432515600003.
[12] Wu, Xinqiang, Xu, Shutao, Zhang, Wenna, Huang, Jindou, Li, Jinzhe, Yu, Bowen, Wei, Yingxu, Liu, Zhongmin. Direct Mechanism of the First Carbon-Carbon Bond Formation in the Methanol-to-Hydrocarbons Process. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION[J]. 2017, 第 1 作者56(31): 9039-9043, https://www.webofscience.com/wos/woscc/full-record/WOS:000424260200016.
[13] Zhang, Mozhi, Xu, Shutao, Li, Jinzhe, Wei, Yingxu, Gong, Yanjun, Chu, Yueying, Zheng, Anmin, Wang, Jinbang, Zhang, Wenna, Wu, Xinqiang, Deng, Feng, Liu, Zhongmin. Methanol to hydrocarbons reaction over H beta zeolites studied by high resolution solid-state NMR spectroscopy: Carbenium ions formation and reaction mechanism. JOURNAL OF CATALYSIS[J]. 2016, 第 10 作者335: 47-57, http://ir.wipm.ac.cn/handle/112942/9198.
[14] 王金棒, 李金哲, 徐舒涛, 郅玉春, 魏迎旭, 何艳丽, 陈景润, 张默之, 王全义, 张雯娜, 武新强, 郭新闻, 刘中民. HZSM-22和SAPO-11催化甲醇转化制烯烃（MTH）反应：酸强度对反应和失活机理的影响. 催化学报[J]. 2015, 第 11 作者36(8): 1392-1402, http://lib.cqvip.com/Qikan/Article/Detail?id=665710049.
[15] Wang Jinbang, Li Jinzhe, Xu Shutao, Zhi Yuchun, Wei Yingxu, He Yanli, Chen Jingrun, Zhang Mozhi, Wang Quanyi, Zhang Wenna, Wu Xinqiang, Guo Xinwen, Liu Zhongmin. HZSM-22和SAPO-11催化甲醇转化制烯烃（MTH）反应：酸强度对反应和失活机理的影响. 催化学报[J]. 2015, 第 11 作者36(8): 1392-1402, http://lib.cqvip.com/Qikan/Article/Detail?id=665710049.
[16] Wang, Jinbang, Li, Jinzhe, Xu, Shutao, Zhi, Yuchun, Wei, Yingxu, He, Yanli, Chen, Jingrun, Zhang, Mozhi, Wang, Quanyi, Zhang, Wenna, Wu, Xinqiang, Guo, Xinwen, Liu, Zhongmin. Methanol to hydrocarbons reaction over HZSM-22 and SAPO-11: Effect of catalyst acid strength on reaction and deactivation mechanism. CHINESE JOURNAL OF CATALYSIS[J]. 2015, 第 11 作者36(8): 1392-1402, http://dx.doi.org/10.1016/S1872-2067(15)60953-6.
[17] 王金棒, 李金哲, 徐舒涛, 郅玉春, 魏迎旭, 何艳丽, 陈景润, 张默之, 王全义, 张雯娜, 武新强, Xinwen Guo, 刘中民. Methanol to hydrocarbons reaction over HZSM-22 and SAPO-11: Effect of catalyst acid strengthon reaction and deactivation mechanism. CHINESE JOURNAL OF CATALYSIS催化学报[J]. 2015, 第 11 作者36: 1392, http://cas-ir.dicp.ac.cn/handle/321008/148156.

   

（ 1 ） 原位谱学技术研究分子筛催化甲醇转化反应诱导期的自催化作用机制, 负责人, 国家任务, 2020-01--2022-12
（ 2 ） “优秀青年博士人才”, 负责人, 研究所自选, 2019-01--2023-12